Yes, you can do a NOT by putting a minus in front of the label. For example:
something = look for pages with a label of "something"
-something = look for pages without a label of "something"
Also, if you need it there's a full explanation of how to do AND and OR in this answer: How do you get only those items with say Label A and Label B and not Label A, Label B AND Label A & B?
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