Is there anyway we can configure Confluence so that when people use the "<Confluence-base-url>/label/.." to look for pages tagged with a certain label - and if that turns up only one page, the user is immediately redirected to the page itself, instead of the "labeled content" page?
Only via a plugin.
I'd imagine you could find an event for that page being viewed. At that point, you could construct your own code to perform some logic (ie how many pages are on the page), and then perform a response (serve a different page, redirect the user, etc).
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